it would seem to be that we are forever destined to be unable to "reach" all the irrationals? By reaching them I mean describing them by some finite operation of integers under the arithmetic operators.
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Correct. Irrationals that satisfy a polynomial
relation (essentially what you're describing) are called algebraic numbers. There are only
countably many of these. Countable means 'is in one-to-one correspondence with the natural numbers'. Sets which are countable are the natural number, the rational numbers, the algebraic integers, and the algebraic numbers, in fact each of these sets is a subset of the later ones in the list.
They constitute only a very small proportion of the real numbers. For instance neither pi nor e are algebraic (in the algebraic integers).
I was basically wondering if this is true or not, and if proofs or more information exists on this. Do we know how large the infinite of the irrationals are compared to the infinite of integers?
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Yes and no. The real numbers have cardinality c (for continuum). Precisely what this is is the subject of the continuum hypothesis and the answer depends on the model of set theory that you use.
(ie, the infinite number of odds should be half the size of the infinite number of integers?)
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For infinite sets size (or cardinality) is defined in terms of functions. There is a bijection between odd and even integers, thus they have the same cardinality. A bijection is a one-to-one correspondence (the maps x to x+1 and x to x-1 are bijections between odd and even integers).
Are there infinities that we can define which are larger than the irrationals?
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Yes. Lots...
Of the top of my head I would guess one could say something like the complex irrationals, but that goes against the spirit of what I am looking for.
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The real and complex numbers have the same cardinality
I guess I mean a series of numbers using just the basic numerical numbers and arithmetic operators.
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By definition these are countable - assuming you mean a finite number of operations.