Suppose you have 6 boxes numbered from 1 to 6. Each time you toss the coin you write the result on a paper and put it in the connected box (the first result in box 1, the second in box 2, etc.). You aim to have three papers on which is written tails and three on which is written heads.
Now if you get three papers of each result, you might choose for example tails. Put all the papers with tails in the boxes. This way you get a way of combining your 3-3 result, because the empty boxes will get the rest of the papers (the ones with heads). So it is enough to put one set of papers to get a solution. that's why you can choose just 3 boxes(experiments) out of 6.
You can think the same for results like 2 tails- 4 heads. This way you can observe that the number you get from choosing 2 experiments out of 6 or 4 out of 6 gives the same result. So you will practically prove that C62 = C64.