In which situations does the equation for torque t=Iα hold?

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The equation for torque, represented as \(\tau = I\ddot{\theta}\), applies specifically to rigid bodies rotating about a fixed axis where the moment of inertia remains constant. This equation can be derived from the angular momentum equation \(\|\vec L\|=I\dot\theta\). The moment of inertia tensor, denoted as \(I_{\mathcal{O}}\), is defined through an integral over the body's volume, and when constrained to a single direction, simplifies to \(\tau_z = (I_{\mathcal{O}})_{zz} \alpha_z\). The equation holds true in scenarios where the moment of inertia does not vary with time.

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The equation ##\|\vec\tau\|=I\ddot\theta## offers a way to calculate the torque acting upon a body which rotates about a fixed axle by using inertia and angular acceleration. This equation can be derived from ##\|\vec L\|=I\dot\theta##.

What I would like to know are the requirements for applying this equation. Thank you.
 
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I don't think your equation as written is correct, since ##\ddot{\theta}## can certainly be negative. Better to write something like ##\tau_z = I \ddot{\theta}_z## or simply ##\tau = I \ddot{\theta}##.

Anyway, suppose a body is undergoing rotation about some fixed point ##\mathcal{O}## (this causes no loss in generality, since any infinitesimal motion can be described as the composition of a translation and a rotation, and by extension any motion can be described by the position of some reference point and the rotation around that reference point).

The moment of inertia tensor at the point ##\mathcal{O}##, which we might call ##I_{\mathcal{O}}##, is defined by an integral ##(I_{\mathcal{O}})_{ij} = \int dV \rho(x_k x_k \delta _{ij} - x_i x_j)##, N.B. summation over repeated indices, over the volume ##\Omega## which comprises the body. The ##\{ x_i \}## coordinates are relative to the origin ##\mathcal{O}##. Then$$L_i = (I_{\mathcal{O}})_{ij} \omega_j$$Now if the moment of inertia is constant during the motion,$$\tau_i = (I_{\mathcal{O}})_{ij} \dot{\omega}_j \equiv (I_{\mathcal{O}})_{ij} \alpha_j$$Furthermore, if the angular acceleration is constrained to only one direction, e.g. perhaps ##\boldsymbol{\alpha} = \alpha \boldsymbol{z} = \ddot{\theta}_z \boldsymbol{z}##, then all the terms in the sum on the RHS drop out except for one, in which case$$\tau_i = (I_{\mathcal{O}})_{iz} \alpha_z$$If you chose your coordinate system to coincide with the principal axes, then ##a\neq b \implies I_{ab} = 0## (i.e. the moment of inertia tensor has diagonal matrix representation), and simply you have$$\tau_z = (I_{\mathcal{O}})_{zz} \alpha_z, \quad \quad \tau_x = \tau_y = 0$$In cases like this it is conventional to rewrite something like ##(I_{\mathcal{O}})_{zz} \equiv (I_{\mathcal{O}})_{z}##.
 
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To answer the question posed in the title of the thread, it holds in situations where the moment of inertia does not have a time dependence. More generally, $$\vec \tau=\frac{d\vec L}{dt}.$$
 
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If ##I## in the OP is meant to be just a scalar this holds for the rotation of a rigid body around a fixed axis. ##I## is then the moment of inertia of the body around this fixed axis.

In general for a rigid body you have a tensor of inertia, explained nicely in ##3, describing the rotation of the body around a point fixed in the body.
 
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