I am not sure about Lorentzian manifolds but for Riemannian manifolds the entire Riemann curvature tensor is determined by the sectional curvatures of tangential 2 planes.
These are the normalized curvatures ,##<R(X,Y)Y,X>/<X,X><Y,Y> - <X,Y>^2##.
The geodesic deviation equation ##D^2J/dt^2 = - R(J(t),c'(t))c'(t)## almost gives you the sectional curvature of the 2 plane spanned by ##J(t)## and ##c'(t)##. One only needs to take the inner product with ##J## and normalize. So for a Riemannian manifold one ought to be able to determine the entire curvature tensor from geodesic deviations. ( Note that sectional curvature is not defined for a degenerate 2 plane on a Lorentzian manifold.)
The variation vector field of a variation through geodesics is always a Jacobi field. That is: it always satisfies the geodesic deviation equation. One can always find a variation through geodesics that has an arbitrary Jacobi field as its variation vector field. This means that one can always compute ##R(J(t),c'(t))c'(t)## at any point along the geodesic in terms of some variation through geodesics. So for a Riemannian manifold the answer to your question is yes.
For a Lorentzian manifold I am not sure since there are degenerate 2 planes. Also the proof that every Jacobi field is the variation vector field of a variation through geodesics depends on the existence of a neighborhood of each point where each point is connected by a unique minimal geodesic. I tried to find a reference on line but without luck. I am sure one of the Relativity experts here would know the answer. In any case, the geodesic deviations ought to tell you a lot about the curvature tensor if not the whole thing. I would be interested to know the answer.