look carefully at the [0, 1, 2, …, N-1]/N I posted above.
Let's say you have 8 samples at sampling rate fs = 8 Hz. The "normal" way you'd label your frequency bins is
[0, 1, 2, …, N-1]/N * fs = [0, 1, 2, …, 7]/8 * 8 Hz = [0, 1, 2, …, 7] Hz.
Since the frequencies wrap around the 8 Hz sampling frequency, these are exactly the same as
[0, 1, 2, …, N/2-1, -N/2, …,-2, -1,]/N * fs = [0, 1, 2, 3, -4, -3, -2, -1]/8 * 8 Hz = [0, 1, 2, 3, -4, -3, -2, -1] Hz.
If you do a quick test, you'll notice that the Fourier coefficients contained in the 1 and -1 Hz bins are just complex conjugates of each other. Similarly for 3, -3 Hz and every other pair of bins. This is because you have a real-valued signal. If you want to so something to your signal but keep it real-valued, you have to maintain this symmetry.
For example, to high pass keeping >= 2 Hz signals, you can zero the 0 Hz and +1, -1 Hz bins and then inverse transform.