How Does ARPES Measure the Lifetime of Injected Photo Holes?

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SUMMARY

Angle-resolved photoemission spectroscopy (ARPES) effectively measures the lifetime of injected photo holes by analyzing the energy distribution curve (EDC) of the ARPES spectrum at specific momentum values. The spectral function, A(k,w), reveals a peak resembling a Lorentzian for Fermi-liquid-type quasiparticles, where the width of this peak indicates the inverse-lifetime of the photo-hole. This method allows researchers to determine the binding energy using the equation Eb = hv - Ekin - W, where hv is photon energy, Ekin is kinetic energy, and W is the work function. The reference to Valla et al., Science v.285, p.2110 (1999) provides foundational context for this analysis.

PREREQUISITES
  • Understanding of angle-resolved photoemission spectroscopy (ARPES)
  • Familiarity with spectral functions and quasiparticles
  • Knowledge of energy distribution curves (EDC)
  • Basic principles of photon energy and work function calculations
NEXT STEPS
  • Study the spectral function A(k,w) in detail
  • Review the methodology of measuring quasiparticle lifetimes in ARPES
  • Examine the implications of Lorentzian peak widths in ARPES data
  • Read Valla et al., Science v.285, p.2110 (1999) for foundational insights
USEFUL FOR

Physicists, materials scientists, and researchers involved in condensed matter physics, particularly those focusing on electronic properties and quasiparticle dynamics using ARPES techniques.

fk08
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Why it is said that ARPES measures the lifetime of the injected photo hole?
When photons with certain energy promote electrons from the initial state to the final state with kinetic energy then by knowing the photon energy one can simply determine the binding energy of the initial state: Eb = hv - Ekin - W(orkfunction).

I do not see the connection to the hole lifetime.
 
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fk08 said:
Why it is said that ARPES measures the lifetime of the injected photo hole?
When photons with certain energy promote electrons from the initial state to the final state with kinetic energy then by knowing the photon energy one can simply determine the binding energy of the initial state: Eb = hv - Ekin - W(orkfunction).

I do not see the connection to the hole lifetime.

You can't get it that way.

What you need to do is look at the energy distribution curve (EDC) of the ARPES spectrum at a particular momentum. This represents what we call the spectral function, A(k,w), at that particular k value. If this is a regular, Fermi-liquid-type quasiparticle, there will be a well-defined peak in the spectrum that closely resembles a Lorentizian. The width of that peak (or full-width at half maximum) corresponds to the inverse-lifetime of the quasiparticle, or photo-hole.

See, for example, Valla et al., Science v.285, p.2110 (1999).

Zz.
 

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