When do fission products get cooler than fuel?

In summary, the conversation discusses the main nuclear fuel, U-235, and its decay process. It is estimated that U-235 causes about 860 MeV worth of damage in its 710 million year half-life. Fission products, even the long-lived ones, are generally cooler than U-235 and pose less of a biological threat. However, transmutation of fission products and neutron capture can result in the production of more dangerous transuranic radioisotopes. There are various plots and data available to show when spent fuel is less radiotoxic than natural uranium ore.
  • #1
snorkack
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Main nuclear fuel is U-235.
Actinium series to stable Pb-207 includes 7 alpha and 4 beta decays. Total energy yield 46,4 MeV.
In the main branch, the 4 beta decays carry around 3 MeV energy. Meaning the alpha decays are about 43 MeV... and they have high biologic effectiveness, around 20. Meaning U-235 does about 860 MeV worth of damage in its 710 million year half-life... about 1200 keV per million years.
When U-235 is fissioned, some daughters are stable. Others are hot but short-lived and promptly decay to stable daughters in 100 years or less half-life
This leaves 7 or so long lived fission products. But even these are beta active... limited total energy, limited biologic effectiveness and limited yield.

Are long lived fission products actually hotter than the original unburned U-235+daughter chain?
 
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  • #2
What do you mean by 'hotter' and 'cooler'? Are you referring to their literal temperature?
 
  • #3
Drakkith said:
What do you mean by 'hotter' and 'cooler'? Are you referring to their literal temperature?
No, as can be seen from my arguments.
"Hotter" as in "more biologically damaging radiation per unit time".
 
  • #4
One could use a spreadsheet and look at the individual and sum of activity (decays/time) and energy deposition (activity * energy/decay) for the longest living fission products, and perhaps the medium fission products, and compare to the activity and energy deposition of 235U. Furthermore, one may consider the specific activity, e.g., per gram of material.

https://en.wikipedia.org/wiki/Long-lived_fission_product#The_7_long-lived_fission_products

However, consider that while 235U is the principal fuel, some fission occurs in 238U from fast neutrons, and perhaps more importantly, both nuclides are transmuted by neutron capture to transuranic radioisotopes, 236Np and 239Pu, respectively, which can also transmute to 237Np and 240Pu, respectively, and so on.

See also, the plot of activities of FP and TU radionuclides:
https://www.titech.ac.jp/english/news/2017/039701

On a related subject matter

Transmutation of long-lived fission products in an advanced nuclear energy system​

https://www.nature.com/articles/s41598-022-06344-y
 
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  • #5
Looks like the long lived fission products, dominated by Tc-99, are 1000 times cooler than uranium, and fission products dominated by Sr-90 get cooler than uranium in 300 years or so... except for the transuranium elements, due to which the radioactivity lasts closer to 10 000 years.
 
  • #6
If you are looking for a general answer of when spent fuel is less radiotoxic than natural uranium ore, there are several plots that you can find on the internet.

For example, this plot shows it will occur in about 200,000 years.
https://en.wikipedia.org/wiki/File:Spent_nuclear_fuel_decay_sievert.jpg

There are other plots you can see by doing a search on "image radioactive decay radiotoxicity"
 
  • #7
snorkack said:
No, as can be seen from my arguments.
"Hotter" as in "more biologically damaging radiation per unit time".
FYI, I couldn't "see" that from your OP, @snorkack, but are you able to share the context for your question? Radiation toxicity depends on many factors such that a 'cooler' element may be more lethal than a 'hotter' one through the circumstances of contact.
 

1. When do fission products start to cool down?

Fission products start to cool down immediately after the fission process occurs. This is because they are highly radioactive and release a large amount of energy in the form of heat. However, the rate of cooling varies depending on the type of fuel and the amount of fission products present.

2. How long does it take for fission products to cool down?

The cooling process for fission products can take anywhere from a few days to several years. This is because different fission products have different half-lives, which is the amount of time it takes for the radioactivity of a substance to decrease by half. Shorter half-lives result in quicker cooling, while longer half-lives result in slower cooling.

3. What factors affect the cooling of fission products?

The main factors that affect the cooling of fission products are the type of fuel used, the amount of fission products produced, and the surrounding environment. Different types of fuel have different compositions and produce varying amounts of fission products. The amount of fission products present also plays a role in the rate of cooling. The surrounding environment can also impact the cooling process, as it can affect the transfer of heat from the fission products.

4. How is the cooling of fission products monitored?

The cooling of fission products is monitored through various methods, such as temperature measurements, radiation detection, and visual inspections. Temperature measurements can give an indication of the heat being released by the fission products. Radiation detection can detect the amount of radioactivity being emitted, which can also indicate the cooling process. Visual inspections can reveal any physical changes in the fission products, such as a decrease in temperature or a change in color.

5. What happens to fission products after they have cooled down?

Once fission products have cooled down, they are typically stored in specialized containers or disposed of in a designated facility. These measures are taken to prevent any potential harm from the remaining radioactivity. In some cases, fission products may also be reprocessed to extract useful materials or to reduce the amount of radioactive waste. The specific disposal or reprocessing methods may vary depending on the country and regulations in place.

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