How Can You Determine the Wavefunction ψ(r) from Electron Density |\psi(r)|^2?

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SUMMARY

The discussion centers on determining the wavefunction ψ(r) from the electron density function |\psi(r)|^2. It is established that while the probability density provides some information, multiple wavefunctions can correspond to the same density, making it impossible to uniquely determine ψ(r) solely from |\psi(r)|^2. For nondegenerate stationary states without spin or angular dependence, the wavefunction can be chosen to be real, allowing for the calculation of ψ(r) by taking the square root of the electron density function.

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I have a 3 dimensional orbital-specfic electron density function ( |[itex]\psi[/itex](r)|2 ) for all relevant r values. How would I go about finding the corresponding [itex]\psi[/itex](r)? I know it would be something related to a Fourier transform, I'm just unsure about how to go about performing it in mathematica or matlab. Can anyone give me any pointers?
 
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You can't. Probability density carries less information than wave function. Many wave functions may lead to the same probability density. Even Fourier can't help.
 
If it's as simple as you're making it sound, with no spin dependence or (θ,φ) dependence, just r dependence, then the wavefunction ψ for a nondegenerate stationary state can always be chosen to be real. (Proof: by time-reversal invariance ψ* is also a solution, so if there's only one solution then ψ = ψ*.) So if that's the case, just take the square root.
 

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