Question about Cumulative Fission Yields

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Discussion Overview

The discussion revolves around cumulative fission yields (CFY) for Gallium isotopes produced from thermal neutron fission of Uranium-233 (U-233). Participants explore the discrepancies in reported values and the implications of neutron energy ranges on these yields, as well as the definitions and sources of data related to CFY.

Discussion Character

  • Exploratory
  • Technical explanation
  • Debate/contested

Main Points Raised

  • Some participants question why thermal U-233 has two different values for Gallium isotopes, suggesting it may relate to the thermal range of neutrons impacting U-233.
  • There is a discussion about the sources of data for cumulative fission yields, with mentions of different databases providing varying values for thermal and fast fissions.
  • One participant notes that the second value for Gallium isotopes might represent uncertainty, referencing data from the European database and the JENDL-4.0 database.
  • Participants express uncertainty regarding the correct definition of CFY, with references to the IAEA definition and a contrasting Wikipedia entry that states it is per 100 fissions.
  • There is mention of the relevance of fast fission in light water reactors (LWR) and molten salt reactors (MSR), with some participants debating the implications of fast neutrons in these contexts.

Areas of Agreement / Disagreement

Participants do not reach a consensus on the reasons for the two values of Gallium isotopes or the correct definition of cumulative fission yields. Multiple competing views remain regarding the interpretation of data and the significance of neutron energy ranges.

Contextual Notes

Participants highlight limitations in the data sources and definitions, noting potential discrepancies between different databases and the need for verification from authoritative sources.

mesa
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So CFY gives the average number of atoms of a specific nuclide produced from a fission directly plus that from the decay of precursors, so why does thermal U233 have two values for Gallium @ 7.192x10^(-8) and 1.0788x10^(-8)? Is this number dependent on the thermal range the neutrons that hit the nucleus of U233?
 
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mesa said:
So CFY gives the average number of atoms of a specific nuclide produced from a fission directly plus that from the decay of precursors, so why does thermal U233 have two values for Gallium @ 7.192x10^(-8) and 1.0788x10^(-8)? Is this number dependent on the thermal range the neutrons that hit the nucleus of U233?
What is the source of the data. Some databases will give a cumulative fission yields for thermal and fast fissions, and some give the fast fission yield at ~1 MeV and/or 14 MeV.
 
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For this topic the interest is in thermal neutron fission, i.e. a MSR, just like a light water solid fuel reactor.
 
Astronuc said:
What is the source of the data. Some databases will give a cumulative fission yields for thermal and fast fissions, and some give the fast fission yield at ~1 MeV and/or 14 MeV.

Just what mheslep said, we are looking at thermal. I got the values for a parent U233 off of this chart for Gallium 69:
http://www-nds.iaea.org/relnsd/vchart/
I don't understand why there are two values there.

I noticed the IAEA definition for CFY's is, "total number of atoms of a specific nuclide produced directly by a fission event and via decay of precursors", (link:http://www-nds.iaea.org/sgnucdat/safeg2008.pdf) but wikepedia says it is per 100 fissions (link:http://www.nucleonica.net/wiki/index.php/Help:Fission_Products_and_Yields ), which is correct?
 
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mesa said:
Just what mheslep said, we are looking at thermal. I got the values for a parent U233 off of this chart for Gallium 69:
http://www-nds.iaea.org/relnsd/vchart/
I don't understand why there are two values there.
The second value should be the uncertainty. These values are from the European database.

From the JENDL-4.0 database (http://wwwndc.jaea.go.jp/cgi-bin/nuclinfo2010a.cgi?31,72,1) for Ga-72 gives:
Code:
Neutron-induced Fission Yields - Cumulative Fission Yield -
Product  Nuclide  Energy(eV)  Fission Yield  Uncertainty(s)
------------------------------------------------------------
Ga- 69    U-233 (T) 2.53e-02   9.397010e-08   4.234410e-08 
Ga- 71    U-233 (T) 2.53e-02   1.617040e-06   7.289880e-07 

Ga- 72   U-233 (T) 2.53e-02   4.163520e-06   2.662330e-06
Ga 69, 71 are stable.
I added 69 from (http://wwwndc.jaea.go.jp/cgi-bin/nuclinfo2010a.cgi?31,69,1)
and 71 from (http://wwwndc.jaea.go.jp/cgi-bin/nuclinfo2010a.cgi?31,71,1)

I noticed the IAEA definition for CFY's is, "total number of atoms of a specific nuclide produced directly by a fission event and via decay of precursors", (link:http://www-nds.iaea.org/sgnucdat/safeg2008.pdf) but wikepedia says it is per 100 fissions (link:http://www.nucleonica.net/wiki/index.php/Help:Fission_Products_and_Yields ), which is correct?
I'd trust the iaea definition, but one should verify with another sources, e.g., US DOE national lab like Brookhaven

mheslep said:
For this topic the interest is in thermal neutron fission, i.e. a MSR, just like a light water solid fuel reactor.
LWR have a fast flux. Fast fission accounts for 8 to 10% of fssions in an LWR, although that is in U-238. Likewise, the MSR will have fast fission. The problematic (n,α) reaction in Ni is from fast neutrons; the (n,α) reaction does not occur at thermal energies.
 
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Astronuc said:
...

LWR have a fast flux. Fast fission accounts for 8 to 10% of fssions in an LWR, although that is in U-238.
Thanks.

Likewise, the MSR will have fast fission.
Would it? Yes there will be fast neutrons, but there would be no U238 in a Th based MSR to fission from fast neutrons.
http://en.wikipedia.org/wiki/Thorium_fuel_cycle#Actinide_wastes
 
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Astronuc said:
The second value should be the uncertainty. These values are from the European database.

From the JENDL-4.0 database (http://wwwndc.jaea.go.jp/cgi-bin/nuclinfo2010a.cgi?31,72,1) for Ga-72 gives:
Code:
Neutron-induced Fission Yields - Cumulative Fission Yield -
Product  Nuclide  Energy(eV)  Fission Yield  Uncertainty(s)
------------------------------------------------------------
Ga- 69    U-233 (T) 2.53e-02   9.397010e-08   4.234410e-08 
Ga- 71    U-233 (T) 2.53e-02   1.617040e-06   7.289880e-07 

Ga- 72   U-233 (T) 2.53e-02   4.163520e-06   2.662330e-06
Ga 69, 71 are stable.
I added 69 from (http://wwwndc.jaea.go.jp/cgi-bin/nuclinfo2010a.cgi?31,69,1)
and 71 from (http://wwwndc.jaea.go.jp/cgi-bin/nuclinfo2010a.cgi?31,71,1)

I'd trust the iaea definition, but one should verify with another sources, e.g., US DOE national lab like Brookhaven

LWR have a fast flux. Fast fission accounts for 8 to 10% of fssions in an LWR, although that is in U-238. Likewise, the MSR will have fast fission. The problematic (n,α) reaction in Ni is from fast neutrons; the (n,α) reaction does not occur at thermal energies.

Uncertainty, very good.
Those values on your table are slightly different from the table I used, should I stick with iaea values or switch to jaea?
 

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