The eye diagram makes my point rather than yours. It's a good tool for the problem it was built for. It's the wrong tool for the one under discussion, which is what "not with a quartz crystal" meant.
Ultrafast imaging doesn't derive frame times from an electronic clock at all. STAMP encodes them in pulse sequence and dispersion:
https://www.nature.com/articles/s41377-018-0044-7. This group,
https://opg.optica.org/josab/abstract.cfm?uri=josab-35-11-2822, set them with mirror-array path-length differences, where 1 µm of path is 3.34 fs. T-CUP and CUSP use temporal shearing and spectral–temporal mapping:
https://www.nature.com/articles/s41467-020-15745-4. What you won't find anywhere are PLLs.
So, no nails here. The main problem to me, as a lowly incoming physics graduate student, is that the bubble nucleation in the bubble chamber might not happen fast enough. What I'm not worried about is image timing, because it's been done.
Not really the point of this thread though, and otherwise the post was relevant to the discussion.