How do scientists work with nonlinear crystals

In summary, scientists say that using a barium borate crystal will decrease the frequency of transmitted laser light by 50%. Scientists tried this experiment with many different laser intensities and found that the conversion efficiency is very low.
  • #1
sciencejournalist00
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When I point a 5 milliwatts red laser at a pile of barium borate crystals, all I get is red speckles of scattered light.
When I point a 100 milliwats blue laser at the same pile of barium borate crystals, I get blue speckles.
When I point a 2000 milliwats green laser at the pile of barium borate crystals, I get green speckles.

Scientists say barium borate should decrease the frequency of transmitted laser light by 50%.

How come spontaneous parametric down conversion I do not observe?

Whether I use a single crystal or more, I get the same result. Speckles of scattered light of the same colour.
 
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  • #2
I bought the crystals a year ago. I tried every day and I got the same result. No frequency change
 
  • #3
Did you ever work with these crystals in the right way? Can you tell which laser intensity you used to get a frequency change
 
  • #4
sciencejournalist00 said:
Did you ever work with these crystals in the right way? Can you tell which laser intensity you used to get a frequency change

Obviously you know even less than I do about this. Start here
 
  • #5
I know how the phenomenon is called and that it requires laser light and special crystals, but I do not understand how to do it practically. What intensity is needed to observe the change of light colour from higher to lower frequency for barium borate?
 
  • #6
https://en.wikipedia.org/wiki/Spontaneous_parametric_down-conversion

In a commonly used SPDC apparatus design, a strong laser beam, termed the "pump" beam, is directed at a BBO (beta-barium borate) crystal. Most of the photons continue straight through the crystal. However, occasionally, some of the photons undergo spontaneous down-conversion with Type II polarization correlation, and the resultant correlated photon pairs have trajectories that are constrained to be within two cones, whose axes are symmetrically arranged relative to the pump beam. Also, due to the conservation of energy, the two photons are always symmetrically located within the cones, relative to the pump beam. Importantly, the trajectories of the photon pairs may exist simultaneously in the two lines where the cones intersect. This results in entanglement of the photon pairs whose polarization are perpendicular
SPDC is stimulated by random vacuum fluctuations, and hence the photon pairs are created at random times. The conversion efficiency is very low, on the order of 1 pair per every 1012 incoming photons.However, if one of the pair (the "signal") is detected at any time then its partner (the "idler") is known to be present. The output of a Type I down converter is a squeezed vacuum that contains only even photon number terms. The output of the Type II down converter is a two-mode squeezed vacuum.


Too low conversion efficiency?
 
  • #7
sciencejournalist00 said:
Did you ever work with these crystals in the right way? Can you tell which laser intensity you used to get a frequency change
If you search the arxiv for "spontaneous parametric down-conversion" you get a lot of papers. Let's take this for example. In the section "experimental results" they state that they use an Omicron LDM405.120.CWA.L.WS laser. Googling this leads to the manufacturer website where the specifications of the laser are stated. So they seem to use 300 mW @405nm (cw).
 
  • #8
Both types of crystals are thin (0.8 mm) in comparison to the Rayleigh length and compared to the transvers eextent of the imaged rings - a requirement for polarization entanglement. As the crystals become thick, which-path information begins to degrade the entanglement because the rings become distinguishable.
cause the rings are elliptical, they no longer perfectly spatially overlap around the entire ring, leading to potential degradation in entanglement-purity, and limiting the
ability to multiplex many channels around the down-conversion ring. Lack of spatial overlap is the most obvious way in which which-path information is
revealed. A smaller overlap integral represents lower entanglement quality because the dierence in spectra between the crystals means it is possible
to distinguish which crystal the photons came from.

http://arxiv.org/pdf/1503.04676v2.pdfSo that is why I got speckles
 
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  • #9
I still get speckles.I tried it over all range of sizes of crystals. I do not get frequency conversion. I really do not know what is happening.

I bet those scientists cannot see the converted photons with their naked eye among unconverted photons. Do they use detectors instead?
 
  • #10
sciencejournalist00 said:
I bet those scientists cannot see the converted photons with their naked eye among unconverted photons. Do they use detectors instead?
That's right.
And even detectors are not sufficient, between sensitive detectors also respond to pretty much every photon that comes by. If you read the actual scientific papers (such as the one that DrChinese pointed you at in your other thread) you'll find a description of the fairly sophisticated methods (often involving coincidence counters) used to pick the detections of converted photons out from the all the rest.
 
  • #11
The downconversion happens with a tiny fraction of the total number of photons. You will never see this with your eye, you need some very effective way to block the light from the laser wavelength to have some chance to see anything.
You might get the conversion, but you just don't see it. A related example: stars are present during daylight, but you also don't see them without specialized equipment.
 
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  • #12
mfb said:
You might get the conversion, but you just don't see it

Right. And if you downconvert red light, you won't see it no matter how much of it you have.
 
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  • #13
sciencejournalist00 said:
I know how the phenomenon is called and that it requires laser light and special crystals, but I do not understand how to do it practically. What intensity is needed to observe the change of light colour from higher to lower frequency for barium borate?

Here is a great reference for the details of creating entangled pairs. This is as basic a "how to" as you will likely find.

http://arxiv.org/abs/quant-ph/0205171

We use polarization-entangled photon pairs to demonstrate quantum nonlocality in an experiment suitable for advanced undergraduates. The photons are produced by spontaneous parametric downconversion using a violet diode laser and two nonlinear crystals. The polarization state of the photons is tunable. Using an entangled state analogous to that described in the Einstein-Podolsky-Rosen ``paradox,'' we demonstrate strong polarization correlations of the entanged photons. Bell's idea of a hidden variable theory is presented by way of an example and compared to the quantum prediction. A test of the Clauser, Horne, Shimony and Holt version of the Bell inequality finds S=2.307±0.035, in clear contradiciton of hidden variable theories. The experiments described can be performed in an afternoon.

And as with the other thread: you seem to be following much of what you are reading but are missing key items. You made a comment about seeing entangled photons with the naked eye, and then fail to ask how you would pick out the 1 in a trillion that meets the entangled criteria in that case. The answer to that is to use filters (to allow only the entangled wavelengths to pass); off-angle collection (as entangled pairs are bent off angle slightly); high intensity; etc.

Also: not all BBo crystals work equally well with all lasers.
 
  • #16
DrChinese said:
Here is a great reference for the details of creating entangled pairs. This is as basic a "how to" as you will likely find.

http://arxiv.org/abs/quant-ph/0205171

We use polarization-entangled photon pairs to demonstrate quantum nonlocality in an experiment suitable for advanced undergraduates. The photons are produced by spontaneous parametric downconversion using a violet diode laser and two nonlinear crystals. The polarization state of the photons is tunable. Using an entangled state analogous to that described in the Einstein-Podolsky-Rosen ``paradox,'' we demonstrate strong polarization correlations of the entanged photons. Bell's idea of a hidden variable theory is presented by way of an example and compared to the quantum prediction. A test of the Clauser, Horne, Shimony and Holt version of the Bell inequality finds S=2.307±0.035, in clear contradiciton of hidden variable theories. The experiments described can be performed in an afternoon.

And as with the other thread: you seem to be following much of what you are reading but are missing key items. You made a comment about seeing entangled photons with the naked eye, and then fail to ask how you would pick out the 1 in a trillion that meets the entangled criteria in that case. The answer to that is to use filters (to allow only the entangled wavelengths to pass); off-angle collection (as entangled pairs are bent off angle slightly); high intensity; etc.

Also: not all BBo crystals work equally well with all lasers.

I got it - I cannot see the converted photons because the intensity of the converted light is very low and cannot be seen with the naked eye. I have to use detectors.

However I wanted to entangle multiple photons at the same time, so if the beam splitter were the only thing needed, I already have a multi-port beam splitter ordered from China that can make photons follow many trajectories at the same time, making them interfere.
 
  • #17
Vanadium 50 said:
Right. And if you downconvert red light, you won't see it no matter how much of it you have.

But infrared can be absorbed by my skin and be felt as heat. However the red laser is also absorbed by my skin and felt as heat, so I don't make any difference between the heat sources.
 
  • #18
I doubt you can feel the heat from a 5 mW laser. (5 mW is ~ 4 calories per hour). Since energy is conserved, downshifting doesn't change the heat produced.
 
  • #19
I have both 5 mW, 100 mW and 2000 mW lasers and I can feel heat from all of them.

Down-converted photons are infrared if the laser is red and I cannot distinguish the heat from infrared light from the heat of red light.
 
  • #20
Even if I get down-converted light, I cannot entangle matter qubits with it because the other non-converted photons will create quantum decoherence and destroy the original entanglement.

However, if I excite matter qubits with lasers and wait for fluorescence light to be emitted and then superpose fluorescence light from multiple matter qubits on a beam splitter and use detectors to herald the outputs, I may get entangled matter.
 
  • #21
sciencejournalist00 said:
However, if I excite matter qubits with lasers and wait for fluorescence light to be emitted and then superpose fluorescence light from multiple matter qubits on a beam splitter and use detectors to herald the outputs, I may get entangled matter.

You are really getting far out there and are mixing up a variety of completely different concepts. Matter qubits? This forum is not for idle speculation. Can I suggest you re-formulate your ideas into simple questions that you can ask? There is a lot of literature out there on the subject of entanglement of matter (ions for example) and you should really read and understand it before you proceed.
 
  • #22
DrChinese said:
You are really getting far out there and are mixing up a variety of completely different concepts. Matter qubits? This forum is not for idle speculation. Can I suggest you re-formulate your ideas into simple questions that you can ask? There is a lot of literature out there on the subject of entanglement of matter (ions for example) and you should really read and understand it before you proceed.

Yes, Professor Weinfurter uses trapped ions as stationary qubits and photons as the flying qubits

https://en.wikipedia.org/wiki/Trapped_ion_quantum_computer
 
  • #23
Here is how I reformulate.

There is an entire discussion on the NakedScientists Magazine forum http://www.thenakedscientists.com/forum/index.php?topic=42384.0
on exactly the same subject and they reach the conclusion they can entangle any two material objects using the same setup as in the ScienceMag article that describes entanglement of two diamonds

 
  • #24
This thread has veered far from the original question (which OP answered for himself back in #6) so it is closed.
 

1. How do scientists select the appropriate nonlinear crystal for a specific experiment?

Scientists use a variety of factors to select the appropriate nonlinear crystal for their experiments. These include the desired wavelength, the intensity of the incident light, and the material properties of the crystal. They also consider the crystal's nonlinear coefficient and its ability to withstand high temperatures and intense light.

2. What techniques do scientists use to characterize the nonlinear properties of crystals?

Scientists use several techniques to characterize the nonlinear properties of crystals. These include the Z-scan technique, which measures the nonlinear refractive index, and the second-harmonic generation (SHG) technique, which measures the nonlinear susceptibility. They may also use spectroscopic methods to study the crystal's optical properties.

3. How do scientists manipulate the nonlinear properties of crystals?

To manipulate the nonlinear properties of crystals, scientists use different methods such as changing the incident light intensity, temperature, or the crystal's orientation. They may also use electric fields or apply pressure to the crystal to induce changes in its nonlinear response.

4. What challenges do scientists face when working with nonlinear crystals?

One of the main challenges scientists face when working with nonlinear crystals is controlling the crystal's temperature. Nonlinear crystals are sensitive to temperature changes, which can affect their nonlinear response. Another challenge is finding a crystal with the desired properties, as not all materials exhibit strong nonlinear effects.

5. How do scientists ensure the accuracy of their results when working with nonlinear crystals?

To ensure the accuracy of their results, scientists perform careful calibration and control experiments. These include measuring the crystal's response without any incident light or using a known reference material. They also repeat their experiments multiple times and compare results to ensure consistency and validity.

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