As an aside: Aluminum salts (some of them) like AlCl3, are extremely toxic. Aluminum is not a required nutrient for mammals AFAIK.
High aluminum levels in water causes neural plaques to form in mammalian brain tissue. Humans can have this happen as well.
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Squirrel incisors have a very hard dentine layer toward the front, and softer dentine in back. As they gnaw something like wood and apparently aluminum metal, it sharpens the incisor, by differential wear. Those teeth grow constantly, and without gnawing activity their jaws would eventually be held wide open. This is why guinea pigs, rabbits, and other related animals that have incisors and diets like squirrels require chew sticks in their cages. Squirrel teeth are extra hard to accommodate a diet that usually includes hard shelled nuts.
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Why they have become aluminum connoisseurs is interesting to say the least. Native aluminum metal does not occur naturally. And humans have been actively smelting aluminum for only a little over 100 years. So the answer has to be along the lines that they "think" it is something else. What they confuse it with, I do not know.
So they may be mineral deficient, but aluminum eating has the potential for toxicity.