Why perfect graphene has nonmagnetic state?

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Discussion Overview

The discussion revolves around the magnetic properties of perfect graphene, particularly why it is considered to be in a nonmagnetic state. Participants explore the implications of its electronic structure and the effects of vacancies on its magnetic characteristics.

Discussion Character

  • Exploratory
  • Technical explanation
  • Debate/contested

Main Points Raised

  • One participant notes that pure graphene has two sub-lattices due to its two carbon atoms and questions why it is nonmagnetic when it has no vacancies.
  • Another participant suggests that the Lewis structure indicates all electrons are paired, implying that graphene should not exhibit magnetic properties.
  • A different participant observes that the electronic band structure shows the Fermi level does not occupy any state, indicating a lack of unpaired electrons.
  • This participant also raises a question about the magnetic states of graphene with two vacancies, proposing two configurations: vacancies on the same sublattice and vacancies on different sublattices, and expresses confusion about the energy implications of these configurations.
  • Another participant explains that in the case of vacancies on the same sublattice, a Lewis structure can be drawn with all paired electrons, while vacancies on different sublattices lead to a diradical state, which is predicted to be ferromagnetic according to Hund's rule.

Areas of Agreement / Disagreement

Participants express differing views on the magnetic properties of graphene, particularly in relation to vacancy configurations and their effects on total energy. The discussion remains unresolved regarding the implications of these configurations on graphene's magnetic state.

Contextual Notes

There are limitations in the discussion regarding the assumptions made about the electronic structure and the definitions of magnetic states. The relationship between vacancy configurations and total energy is not fully explored.

Hyeonyeong Kim
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I'm major in chemistry my undergraduate.. and not good at Physics, Solid states... etc.

I know pure graphene has two sub-lattice because it has two carbon atoms.. and something basic properties.

then, why perfect graphene(no vacancy) is in nonmagnetic?
 
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Already its Lewis structure should tell you that all electrons are paired. So why do you expect it to be magnetic?
 
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yes.. that is reasonable.

when I saw the electronic band structure, I could see fermi level does not put on any state.

it say there is not unpaired electron. sorry. I think I had to post more better question.Actually I want to know, when graphene has two vacancy, graphene can get the two vacancy configuration.

1. same sublattice, 2. different sublattice.

I knew there magnetic trend..
1 : ferromagnetic state
2 : nonmagnetic state

I couldn't understand in case of 2, why graphene can get more low total energy?In case of 2, I thought my question has something relation with my first question. that is my mistake.

sorry for my low english level.
 
In case 2 you can draw a Lewis structure where all electrons are paired up, in cade 1 you cannot but get a diradical which by Hund's rule will be a triplet, i.e. ferromagnetic.
 

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