The first equation you have after the heading "Loop B E F C" is:
2v = 6ΩI2 + 1ΩI1(I2-I1)
The I1 in red shouldn't be there. Then next you have:
2V = 1ΩI1 + 7ΩI2 but it should be:
2V = -1ΩI1 + 7ΩI2
Next you have :
3V = 4ΩI1 - 1ΩI2 which you brought down from Loop A B C E; it is correct.
But next you rewrote equation (2) introducing a typo. The coefficient of I1 should be -1Ω (although you had +1Ω; you didn't even copy what you had correctly, but it was wrong anyway. But, at the very least you should be able to copy it without introducing a typo). You have:
2V = -4ΩI1 + 7ΩI2
but it should be:
2V = -1ΩI1 + 7ΩI2
Then you copied equation 1 again:
3V = 4ΩI1 - 1ΩI2
Next, you multiplied your incorrect version of equation 2 by 4:
8V = -16ΩI1 + 28ΩI2
but it should actually be:
8V = -4ΩI1 + 28ΩI2
Apparently, what you did at the end was to add these two equations:
3V = 4ΩI1 - 1ΩI2
8V = -16ΩI1 + 28ΩI2
and got as a result:
11V = 27ΩI2
But if you had done the algebra correctly, you would have gotten:
11V = -12ΩI1 + 27ΩI2
which would have given you a wrong answer.
The two equations you should have added are:
3V = 4ΩI1 - 1ΩI2 This is the correct equation (1) from Loop A B C D
8V = -4ΩI1 + 28ΩI2 This is the correct equation (2)
Now, if you add these two equations, you get:
11V = 27ΩI2 which is correct. You somehow got this even though your algebra was incorrect.
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Next, you aren't keeping track of your units properly.
Under the heading "Sub I2 into equation (1)", you have:
3V = 4ΩI1 - 1ΩI2 (0.407a)
which then becomes:
3V = 4ΩI1 - 0.407a
but the second term on the right hand side isn't amps; you got it by multiplying 1Ω times .407 amps which gives .407 volts, not .407 amps.
The units problem still exists in the next equation:
3V + 0.407a = 4ΩI1
It should be 3V + 0.407V = 4ΩI1
Then you would have:
I1 = 3V/4Ω + 0.407V/4Ω = 0.851a
I think you need to practice your algebra skills some more, and exercise greater care with your units.