Xylourgos said:
Dear Astronuc (or others)
Several questions regarding the spent fuel rods;
If water is added to the dried out storage tank, will future radioactive emissions be contained? even if the protective jacket is breached?
If the fuel rods breach, they release fission product gases, Kr and Xe, and volatiles such as Br and I, and possibly Cs. Cs, like Na or K, is more likely to dissolve in water. Other fission products, which are more or less solid, would be retained in the fuel matrix or dissolve in water. Some UO2 may oxidize, a process occurring mostly along grain boundaries (grain size on the order of microns), and particles of fuel, either single grains or groups, can fall out of the fuel into the water. Single grains or lightest particle may become dust.
Assuming that the outer protective jacket of the spent fuel rods have been damaged/melted, when water is added to the pond in order to cool the reaction, will the water itself be contaminated by the released radioactivity?
Yes, some fission products will dissolve in water, and some particulates will migrate into the water.
If this is the case, how will the contaminated water eventually be collected and contained?
Very good question. I would expect that a circulation system would be established, and the particles collected on filters. The challenge will be the volume of water, the surface areas, and the mass of fuel to be collected. Not only is the SFP affected, but also the primary and secondary containments.
In the case that the water evaporates due to the absorption of the heat, will the evaporated water vapor be radioactive?
Noble gases and some volatiles can be carried with the steam plume.
What are the decay products in the spent fuel rods? Do they have long half-lifes?
I'll post a chart of fission products in a bit, maybe in a separate thread. Some decay in seconds, others in the fuel matrix in thousands or millions of years. Short-lived FPs decay away rapidly. In 10 half-lives, activity drops by a factor of 1000, in 20 HL, activity drops by a factor of 1M, and in 30 HL, activity drops by a factor of 1 Billion. Basically the activity drops by 2^N, where N is the number of HL.
I attach a link that illustrates the location of the storage tank. The tank is not located on the roof. However, it is located in the upper part of the concrete structure. Can anyone explain why the tanks are not designed to be built into the lower ground level? Seems to me to be a more prudent design to have the tank supported on the ground.
http://www.npr.org/2011/03/15/134569191/spent-fuel-rods-now-a-concern-at-nuclear-plant
The spent fuel pool is located near the reactor cavity so that discharge fuel can be removed under the cover of water from the reactor core to the spent fuel pool. The fuel to be reused/reinserted in the next cycle may also be placed temporarily in the SFP. The SFP is an interim storage to allow cooldown (thermally and radiologically) of the fuel until it is placed in dry storage. In some modern containments, the spent fuel pool is placed in a separate, but well protected area.
It would seem that a relatively small volume of concrete could effectively cover the tank to prevent radioactive leakage - say 2-3,000 m3. Would this be an effective way to contain the radioactive leakage?
Possibly. However, it would complicate longer term plans to decontaminate and decomission the facility. It would also increase the load on the containment below the pool, and possibly increase the risk of structural failure, particularly in case of another significant seismic event.
Experts knock notion of burying Japanese reactors
http://news.yahoo.com/s/ap/20110318/ap_on_sc/us_japan_nuclear_burial
Thanks in advance for answering my questions.
You're welcome.
I wish good luck to those on the ground containing the problem!
Me too!
FYI -
SUBJECT: DRAFT FINAL TECHNICAL STUDY OF SPENT FUEL POOL ACCIDENT RISK AT DECOMMISSIONING NUCLEAR POWER PLANTS
http://www.nrc.gov/reading-rm/doc-collections/acrs/letters/2000/4711885.html
Fact Sheet on NRC Review of Paper on Reducing Hazards from Stored Spent Nuclear Fuel
http://www.nrc.gov/reading-rm/doc-collections/fact-sheets/reducing-hazards-spent-fuel.html
Safety and Security of Commercial Spent Nuclear Fuel Storage: Public Report (2006)
Board on Radioactive Waste Management (BRWM)
http://www.nap.edu/openbook.php?record_id=11263
"Radiological Terrorism: Sabotage of Spent Fuel Pools"
Journal Article, INESAP: International Network of Engineers and Scientists Against Proliferation, issue 22, pages 75-78
http://belfercenter.ksg.harvard.edu/publication/364/radiological_terrorism.html
Yay Mothers for Peace!
http://mothersforpeace.org/data/20010201Nureg1738Pdf/at_download/file (it may take a while to download) - 18.4 MB
Alternatively http://mothersforpeace.org/data/20010201Nureg1738Pdf/view