Nice article, Shayan.
I've pondered the use of entropy in QM for many years and still don't feel I've really got the hang of it too well. I've always found Shannon's formulation and von Neumann's quantum generalization of it to be rather elegant and fundamental. For me, though, it isn't the entanglement entropy, per se, that's important but rather the ##mutual## information - of course for pure states of bipartite systems the entanglement entropy and mutual information are proportional to one another.
If we have 2 quantum systems ##A## and ##B## with total entropy ##S## and reduced entropies ##S_A## and ##S_B## then they are related by the Araki-Lieb inequality $$ \left| S_A - S_B \right| \leq S \leq S_A + S_B $$The RHS of this inequality is of course that of classical systems - the entropy of the whole must be less than or equal to the sum of the entropies of its constituents. The LHS is where the quantum magic comes in. For pure states of the combined ##AB## system the von Neumann entropy is zero so that in any (combined) pure state of 2 systems the quantum entropies of the 2 component pieces are equal, that is, ##S_A = S_B##.
The mutual information is a measure of the 'information content' of the correlation. In other words, if we only did measurements on the 2 systems alone it is the amount of information we would miss by not considering joint properties. With the mutual information defined as ##I = S_A + S_B - S## then using the AL inequality it's easy to show that $$ I \leq 2 \text {inf} \left\{ S_A , S_B \right\} $$The maximum is obtained when the smaller component system is 'maximally' mixed. The classical version of the AL inequality would be $$ \rm {sup} \left\{ S_A , S_B \right\} \leq S \leq S_A + S_B $$ so that the total entropy, classically, can't be less than the entropy of either of its constituents.
For EM fields, the 2-mode squeezed state can be considered to be a purification of the single mode thermal state - and the mutual information formalism tells us that the two-mode squeezed state is the most strongly correlated state of 2 modes of the EM field, subject to a mean energy constraint.
If we generalize this measure of correlation to multipartite quantum systems (eg, ## I = S_A + S_B + S_C - S##) then some nice general properties can be derived for the evolution of correlations under unitary evolutions using only very elementary methods. The nice thing about this generalization to multipartite systems is that the mutual information is the only sensible measure that satisfies some reasonable properties - for example, if we had 2 uncorrelated (unentangled) systems ##A## and ##B##, each comprised of component parts, then any measure of correlation of the combined ##AB## system should just give the sum of the amount of correlation ##within## each of ##A## and ##B##.
I still think there's more insight to be gained from the use of entropy/information in QM - but it will take a more talented person than me to figure it out
