The picture that emerged from a variety of official data points to quite a collection of significant releases over a number of days early on. The releases that seem to be responsible for the plumes that caused significant land pollution were probably from reactor 1 and then later a much more significant one from reactor 2, which is blamed for around 90% of the total radioactive release into the air.
What I cannot say with any certainty is how much of this stuff came from vent stack rather than more directly from the reactor, turbine or waste processing buildings of each reactor after containment damage and explosions. Early contamination data from before reactor 1 explosion certainly points to some radioactive material having traveled off-site before the explosion, so I think its probably reasonable to expect that venting had a notable impact in this regard.
As for reactor 2, they had a lot of trouble trying to get venting procedures to work, so the picture as to whether venting happened successfully, to what extent, and at what time, is less than complete. And despite the official estimations for radioactive release putting so much blame on reactor 2, we never really got much more detail from company, government or media about this. But if we recall how the news of the suspected explosion near the suppression chamber was treated when it happened, it was considered a big deal and so it would be reasonable to think that this event, rather than venting via stack, caused a lot of the reactor 2 release. But I cannot rule out a large amount coming from the stack via venting either, not enough information & visual evidence to be sure.
I think Reactor 3 explosion stuff was lately carried away from land due to wind direction at the time, and I have not studied venting activity for reactor 3 or tried to connect it to times when site radiation levels rose.
Official data also shows that significant releases (albeit several orders of magnitude less than the peak release rate) continued for much of March, and it is possible that some of this was due to further venting.
The chart of estimated release rates over time may be of help when trying to get our heads round this stuff, or quite the opposite as it kills the simplified version of events: