How can we efficiently dry metallic nanoparticles

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Discussion Overview

The discussion revolves around methods for efficiently drying metallic nanoparticles synthesized in water while preserving their shape and preventing aggregation. Participants explore various techniques and considerations related to the drying process, including the potential for synthesizing nanoparticles directly in an organic phase.

Discussion Character

  • Exploratory
  • Technical explanation
  • Debate/contested

Main Points Raised

  • One participant suggests heating in a vacuum as a potential method for drying the nanoparticles.
  • Another participant notes that metallic nanoparticles are sensitive to higher temperatures and mentions difficulties with drying in a rotary evaporator, where the nanoparticles remain stuck in the vial.
  • A participant discusses the role of vapor pressure and suggests that sticking to the vial may be influenced by the solution's composition and Van der Waals forces.
  • There is a proposal for using a DIY miniature fluidized bed to blow air through a filter membrane to facilitate drying.
  • One participant emphasizes the need to avoid agglomeration while drying, as the goal is to redissolve the nanoparticles in organic solvents.
  • Questions are raised about the type of metal used for the nanoparticles and the potential use of surfactants to aid in transferring them to the organic phase.
  • Another participant mentions that even with the addition of organic solvents, nanoparticles may have an affinity for water, complicating the drying process.
  • There is a discussion about the use of long-chain alkylthiols to moderate the growth of gold nanoparticles, with a request for references on this topic.
  • A reference to a paper from the Whitesides group on gold-thiol self-assembled monolayers is provided as a resource for further exploration.

Areas of Agreement / Disagreement

Participants express various methods and considerations for drying metallic nanoparticles, but there is no consensus on the most effective approach. Multiple competing views and techniques are presented, indicating an unresolved discussion.

Contextual Notes

Participants mention specific challenges related to the drying process, such as the sensitivity of nanoparticles to temperature and their tendency to stick to vials. There are also unresolved questions regarding the role of surfactants and the specific conditions needed for successful transfer to organic solvents.

nadaben
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hello everyone

i wonder if someone can help me to dry completely metallic nanoparticles synthesized in water
while maintaining their shape (without aggregation).or if there is a way to synthesize them directly in organic phase
 
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normally metallic nanoparticles are sensitive to higher temperatures.. i tried to dry them in rotary evaporator but they remains sticked in the vial
 
It's about vapor pressure. If they are metallic they can survive some temperature elevation and it may not take much. Sticking to the vial may be a function of what is in solution with them and or something as simple a Van der Waals forces.

Another approach might be the use of a desiccant.
 
DIY miniature fluidised bed . Air blown . Optionally other gasses or solvent vapour .

Basically blow air the wrong way through filter membrane .
 
The nanoparticles are prepared in water ! I have no other products in the solution.. the goal is to dry and redissolve them in organic solvents so I must avoid agglomerating them while drying
 
I don't claim to be even mildly familiar with nano-particles (outside of some experience with polystyrene micro spheres suspended in water). Would it be possible to add the aqueous suspension into your organic solvent then remove the excess water?
 
First question: what metal?
Second question: do you not want to cap the NPs with a surfactant?
nadaben said:
hello everyone

i wonder if someone can help me to dry completely metallic nanoparticles synthesized in water
while maintaining their shape (without aggregation).or if there is a way to synthesize them directly in organic phase
 
Even if we add the organic solvent nanoparticles have an affinity to water so they remain in the aqueous phase
Metal are gold or silver...what is the role of the surfactant? Is it to transfer them to the organic phase? In this case I've tried this method but it doesn't work for my solvent( chlorobenzene) and for bigger sizes of nanoparticles
 
  • #10
So you don't use something like a long-chain alkylthiol to moderate AuNP growth?
 
  • #11
No actually i didn't try! Do you have references in this way?
 
  • #12
https://gmwgroup.harvard.edu/pubs/pdf/508.pdf
This is one of the early papers from the Whitesides group. They specialized in gold-thiol SAMs for a while back in the 90s-2000s.
 
  • #13
Thank u so much ! It's a very important work .. i should look for its details ! If u have any other ideas or references please share
 

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