I wanted to give some information about results and measurement methods for iodine-131. The french CRIIRAD (which is a laboratory specialized in nuclear monitoring and is independant from french autorities) has published an article explaining how activity of this element in the air (in Bq/m3) has to measured. The important thing to remember is that some measurements methods (and more precisely some sampling methods) only show part of the total activity of the element in the air (which can then go to the soils and the fields when it's raining for example).
Iodine-131 can be present in the air either as:
a) particulates, which can be sampled with appropriate filters,
b) but it can also be present in the air under gazeous forms, and these WON'T BE CAPTURED BY THE SAME FILTERS, BUT NEED A SPECIFIC PROTOCOL OF SAMPLING WITH AIR CARTRIDGES containing charcoal.
IT IS IMPORTANT TO KNOW THAT THIS SECOND FORM (GAZEOUS IODINE 131) CAN BE 3 TO 14 TIMES MORE IMPORTANT THAN THE PARTICULATES FORM OF IODINE-131.
CRIIRAD is producing a report in which they show the example of recent measurements done by EPA on the air in the US after the fukushima accident.
The US report is here:
http://www.criirad.org/actualites/dossier2011/japon/radnet.pdf
I extract the paragraphs describing the two sampling methods used:
Results are presented from two types of air sampling: air canisters and air filters.
• Air Cartridge Sampling: RadNet deployable monitors pass air through a canister that contains charcoal. The cartridges collect radioactive particles and gases in much the same way that a home charcoal air filter traps cooking odors. The canisters are sent to an EPA laboratory for a sensitive laboratory analysis which can detect any radionuclides in the sample. The date on the table is the day that the canister was taken off the sampler.
• Filter Sampling: RadNet fixed or deployable monitors pass air through a filter which traps particulates. The filter is sent to an EPA laboratory for a sensitive laboratory analysis which can detect any radionuclides present. The date on the table is the day that the filter was taken off the sampler for analysis.
You can see in this other document (in french), in the colored results table (going down in the page):
http://94.23.16.204/criirad_telechargement_pdf/eau_de_pluie_iode_131.pdf
that the ratio between gazeous form/particulates form of iodine-131 can vary from 3 to 14 (for example, there was 14 times more gazeous form of iodine in the air at Dutch Harbour than there was in particulates form).
CRIIRAD is pushing a lot the information on this subject because in France the autorities give a lot of data about the iodine-131 activity in the air (through a network called teleray) BUT these numbers are based on a sampling method with filters which can just measure particulate form of iodine. So the numbers given can in fact be several times lower than reality because this network doesn't take into account gazeous forms.
Don't know how it is done in Japan but i thought this had to be presented here and known by people for correctly assessing the total activity of iodine-131 in the air. If you see activities of iodine-131 in Bq/m3, check or ask how measurements were done and if all the forms of iodine-131 (particulates AND gaz) have been sampled.
Measurements are not always an easy matter, this is an example of its tricks and of its complexity.